• Soil Washing Technology for Sr and Cs-contaminated Soil Near Nuclear Power Plants using Calcium and Potassium Based Solutions
  • Hojae Song1·Kyoungphile Nam1*

  • 1Department of Civil and Environmental Engineering, Seoul National University, Gwanak-ro 1, Gwanak-gu, Seoul 08826, Korea

  • 칼슘 및 칼륨 용액을 이용한 원자력발전소 주변 스트론튬과 세슘 오염토양 세척기술 연구
  • 송호재1·남경필1*

  • 1서울대학교 건설환경공학부

  • This article is an open access article distributed under the terms of the Creative Commons Attribution Non-Commercial License (http://creativecommons.org/licenses/by-nc/4.0) which permits unrestricted non-commercial use, distribution, and reproduction in any medium, provided the original work is properly cited.

References
  • 1. Abumaizar, R.J. and Smith, E.H., 1999, Heavy metal contaminants removal by soil washing, Jounral of Hazardous Materials, 70(1-2), 71-86.
  •  
  • 2. Andrade, M., Prasher, S., and Hendershot, W., 2007. Optimizing the molarity of a EDTA washing solution for saturated-soil remediation of trace metal contaminated soils, Environmental Pollution, 147(3), 781-790.
  •  
  • 3. Apelblat, A., 2014, Citric acid, Springer.
  •  
  • 4. Bache, B.W., 1976, The measurement of cation exchange capacity of soils, Journal of the Science of Food and Agriculture, 27(3), 273-280.
  •  
  • 5. Baek, K.T., Kim, D.H., Seo, C.I., Yang, J.S., and Lee, J.Y., 2007, Remediation of pb-contaminated soil by soil washing using hdrochloric acid, Journal of Soil and Groundwater Environment, 12(3), 17-22.
  •  
  • 6. Becker, P., 1983, Phosphates and phosphoric acid, Marcel Dekker, Inc.
  •  
  • 7. Bunde, R., Rosentreter, J., Liszewski, M., Hemming, C., and Welhan, J., 1997, Effects of calcium and magnesium on strontium distribution coefficients, Environmental Geology, 32, 219-229.
  •  
  • 8. Burger, A. and Lichtscheidl, I., 2019, Strontium in the environment: Review about reactions of plants towards stable and radioactive strontium isotopes, Science of the Total Environment,653, 1458-1512.
  •  
  • 9. Cabrera, W.E., Schrooten, I., De Broe, M.E., and d'Haese, P.C., 1999, Strontium and bone, Journal of Bone and Mineral Research, 14(5), 661-668.
  •  
  • 10. Cheong, D.C., Lee, J.H., and Choi, S.I., 1997, Application of soil washing technology to the soil contaminated by heavy metals, J. of KoSES, 2.2, 53-60.
  •  
  • 11. Comar, C.L., Russell, R.S., and Wasserman, R.H., 1957, Strontium-calcium movement from soil to man, Science, 126(3272), 485-492.
  •  
  • 12. Dye, J.L., 1979, Compounds of alkali-metal anions, Angewandte Chemie-International Edition in English, 18(8), 587-598.
  •  
  • 13. EPA, U., 1996, Method 3052: Microwave assisted acid digestion of siliceous and organically based matrices.
  •  
  • 14. Fiume, M.M., Heldreth, B.A., Bergfeld, W.F., Belsito, D.V., Hill, R.A., Klaassen, C.D., Liebler, D.C., Marks Jr, J.G., Shank, R.C., and Slaga, T.J., 2014, Safety assessment of citric acid, inorganic citrate salts, and alkyl citrate esters as used in cosmetics, International Journal of Toxicology,33, 16S-46S.
  •  
  • 15. Fuhrmann, M., Lasat, M.M., Ebbs, S.D., Kochian, L.V., and Cornish, J., 2002, Uptake of cesium‐137 and strontium‐90 from contaminated soil by three plant species; application to phytoremediation, Journal of Environmental Quality, 31(3), 904-909.
  •  
  • 16. George, R., Joy, V., Aiswarya, S., and Jacob, P., 2014. Treatment methods for contaminated soils-translating science into practice, International Journal of Education and Applied Research, 4, 17-19.
  •  
  • 17. Graham, T., 1843, Elements of Chemistry: Including the Applications of the Science in the Arts, Lea & Blanchard.
  •  
  • 18. Greenwood, N.N. and Earnshaw, A., 2012, Chemistry of the Elements, Elsevier.
  •  
  • 19. Kabata-Pendias, A., 1993, Behavioural properties of trace metals in soils, Applied Geochemistry, 8, 3-9.
  •  
  • 20. Lanigan, R.S. and Yamarik, T.A., 2002, Final report on the safety assessment of EDTA, calcium disodium EDTA, diammonium EDTA, dipotassium EDTA, disodium EDTA, TEA-EDTA, tetrasodium EDTA, tripotassium EDTA, trisodium EDTA, HEDTA, and trisodium HEDTA, International Journal of Toxicology,21(Supple 2), 95-142.
  •  
  • 21. Lee, S.H., Kim, E.Y., Seo, S.K., Kim, G.B., Kim, J.H., and Lee, J.K., 2008, Remediation of heavy metal contamination in OBOD site with soil washing: selection of extractants, Journal of Soil and Groundwater Environment, 13(2), 44-53.
  •  
  • 22. Lee, S.O., Tran, T., Jung, B.H., Kim, S.J., and Kim, M.J., 2007, Dissolution of iron oxide using oxalic acid, Hydrometallurgy, 87(3-4), 91-99.
  •  
  • 23. Lenoble, V., Laclautre, C., Deluchat, V., Serpaud, B., and Bollinger, J.-C., 2005, Arsenic removal by adsorption on iron (III) phosphate, Journal of Hazardous Materials, 123(1-3), 262-268.
  •  
  • 24. Li, C., Zhou, K., Qin, W., Tian, C., Qi, M., Yan, X., and Han, W., 2019, A review on heavy metals contamination in soil: effects, sources, and remediation techniques, Soil and Sediment Contamination: An International Journal, 28(4), 380-394.
  •  
  • 25. Lukšienė, B., Marčiulionienė, D., Rožkov, A., Gudelis, A., Holm, E., and Galvonaitė, A., 2012, Distribution of artificial gamma-ray emitting radionuclide activity concentration in the top soil in the vicinity of the Ignalina Nuclear Power Plant and other regions in Lithuania, Science of the Total Environment, 439, 96-105.
  •  
  • 26. Ma, B., Oh, S., Shin, W.S., and Choi, S.-J., 2011, Removal of Co2+, Sr2+ and Cs+ from aqueous solution by phosphate-modified montmorillonite (PMM), Desalination, 276(1-3), 336-346.
  •  
  • 27. Oustan, S., Heidari, S., Neyshabouri, M., Reyhanitabar, A., and Bybordi, A., 2011, Removal of heavy metals from a contaminated calcareous soil using oxalic and acetic acids as chelating agents, International Conference on Environment Science and Engineering IPCBEE, pp. 152-155.
  •  
  • 28. Pamukcu, S. and Wittle, J.K., 1992, Electrokinetic Removal of Selected Heavy-Metals from Soil, Environmental Progress, 11(3), 241-250.
  •  
  • 29. Paolieri, M., 2017, Ferdinand Münz: EDTA and 40 years of inventions, Bull. Hist. Chem., 42(2), 133-140.
  •  
  • 30. Pelc, H., Elvers, B., and Hawkins, S., 2005, Ullmann¡¯s encyclopedia of industrial chemistry, Wiley-VCH Verlag GmbH & Co. KGaA Weinheim.
  •  
  • 31. Schumacher, B.A., 2002, Methods for the determination of total organic carbon (TOC) in soils and sediments.
  •  
  • 32. Seo, S.K., Lee, S.H., Son, J.H., and Son, J.H., 2008 Application of a full scale soil washing process for the remediation of contaminated soil around an abandoned mine, Journal of Soil and Groundwater Environment, 13(2), 70-75.
  •  
  • 33. Singer, M.J. and Janitzky, P., 1986, Field and laboratory procedures used in a soil chronosequence study, Department of the Interior, US Geological Survey.
  •  
  • 34. Singh, S., Eapen, S., Thorat, V., Kaushik, C.P., Raj, K., and D¡¯Souza, S.F., 2008, Phytoremediation of 137cesium and 90strontium from solutions and low-level nuclear waste by Vetiveria zizanoides, Ecotoxicology and Environmental Safety, 69(2), 306-311.
  •  
  • 35. Solanki, A.B., Parikh, J.R., and Parikh, R.H., 2007, Formulation and optimization of piroxicam proniosomes by 3-factor, 3-level Box-Behnken design, Aaps Pharmscitech, 8(43).
  •  
  • 36. Song, H., Chung, H., and Nam, K., 2021a, Effect of monovalent and divalent ion solutions as washing agents on the removal of Sr and Cs from soil near a nuclear power plant, Journal of Hazardous Materials, 412, 125165.
  •  
  • 37. Song, H., Chung, H., and Nam, K., 2021b, Response surface modeling with Box-Behnken design for strontium removal from soil by calcium-based solution, Environmental Pollution, 274, 116577.
  •  
  • 38. Su, C., 2014, A review on heavy metal contamination in the soil worldwide: Situation, impact and remediation techniques, Environmental Skeptics and Critics, 3(2), 24-38.
  •  
  • 39. Sumner, M.E., 1994, Measurement of Soil-Ph - Problems and Solutions, Communications in Soil Science and Plant Analysis, 25(7-8), 859-879.
  •  
  • 40. Tessier, A., Campbell, P.G., and Bisson, M., 1979, Sequential extraction procedure for the speciation of particulate trace metals, Anal. Chem., 51(7), 844-851.
  •  
  • 41. Van Bergeijk, K.E., Noordijk, H., Lembrechts, J., and Frissel, M.J., 1992, Influence of pH, soil type and soil organic matter content on soil-to-plant transfer of radiocesium and-strontium as analyzed by a nonparametric method, Journal of Environmental Radioactivity, 15(3), 265-276.
  •  
  • 42. Vilčiauskas, L., Tuckerman, M.E., Bester, G., Paddison, S.J., and Kreuer, K.-D., 2012, The mechanism of proton conduction in phosphoric acid, Nature Chemistry, 4, 461.
  •  
  • 43. Wei, M., Chen, J., and Wang, X., 2016, Removal of arsenic and cadmium with sequential soil washing techniques using Na2EDTA, oxalic and phosphoric acid: optimization conditions, removal effectiveness and ecological risks, Chemosphere, 156, 252-261.
  •  
  • 44. Williams, L.B. and Ferrell, R.E., 1991, Ammonium substitution in illite during maturation of organic-matter, Clays and Clay Minerals, 39, 400-408.
  •  
  • 45. Wuana, R.A. and Okieimen, F.E., 2011, Heavy metals in contaminated soils: a review of sources, chemistry, risks and best available strategies for remediation, Isrn Ecology 2011.
  •  
  • 46. Yetilmezsoy, K., Demirel, S., and Vanderbei, R.J., 2009, Response surface modeling of Pb (II) removal from aqueous solution by Pistacia vera L.: Box-Behnken experimental design, Journal of Hazardous Materials, 171(1-3), 551-562.
  •  
  • 47. Zhang, W., Huang, H., Tan, F., Wang, H., and Qiu, R., 2010, Influence of EDTA washing on the species and mobility of heavy metals residual in soils, Journal of Hazardous Materials, 173(1-3), 369-376.
  •  

This Article

  • 2022; 27(2): 76-86

    Published on Apr 30, 2022

  • 10.7857/JSGE.2022.27.2.076
  • Received on Feb 21, 2022
  • Revised on Mar 2, 2022
  • Accepted on Apr 11, 2022

Correspondence to

  • Kyoungphile Nam
  • Department of Civil and Environmental Engineering, Seoul National University, Gwanak-ro 1, Gwanak-gu, Seoul 08826, Korea

  • E-mail: kpnam@snu.ac.kr